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题名: New Duclauxamide from Penicillium manginii YIM PH30375 and Structure Revision of the Duclauxin Family
作者: Cao, Pei; Yang, Jing; Miao, Cui-Ping; Yan, Yijun; Ma, Ya-Tuan; Li, Xiao-Nian; Zhao, Li-Xing; null(黄胜雄)
刊名: ORGANIC LETTERS
英文摘要: Duclauxamide A1 (1), a new polyketide-derived heptacyclic oligophenalenone dimer with a N-2-hydroxyethyl moiety, was isolated from Penicillium manginii YIM PH30375. Spectroscopic analysis, X-ray single crystal diffraction, and C-13 NMR DFT calculations confirmed that compound 1 and other duclauxin analogues possess the unified S configuration at C-9', which corrects a long-standing misrepresentation of duclauxins as C-9'R epimers. A plausible biosynthetic pathway for duclauxins is proposed on the basis of previous acetate labeling results for duclauxin and sclerodin.
出版日期: 2015-03-06
卷号: 17, 期号:5, 页码:1146-1149
DOI标识: 10.1021/acs.orglett.5b00081
语种: 英语
收录类别: SCI
学科分类: Chemistry, Organic
Citation statistics:
内容类型: 期刊论文
URI标识: http://ir.kib.ac.cn/handle/151853/20576
Appears in Collections:植物化学与西部植物资源持续利用国家重点实验室_期刊论文

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