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题名: Catalytic asymmetric formal total synthesis of (+)-dichroanone and (+)-taiwaniaquinone H
作者: Li, Liang-Qun1, 2, 3; Li, Ming-Ming2; Chen, Dong2, 3; Liu, Hao-Miao2, 3; Geng, Hui-Chun2, 3; Lin, Jun1; null(秦红波)2
刊名: TETRAHEDRON LETTERS
关键词: Stereoselective formal synthesis ; (+)-Dichroanone ; (+)-Taiwaniaquinone H ; Conjugate addition ; Reetz reagent
英文摘要: Catalytic asymmetric formal total synthesis of (+)-dichroanone and (+)-taiwaniaquinone H has been achieved. Key step involved construction of all-carbon quaternary carbon by palladium-catalyzed conjugate addition of arylboronic acid to 3-methyl cyclohexenone. Furthermore, a new approach to build [6-5-6] tricyclic backbone via formyl introduction and subsequent aldol-type condensation was also explored. (C) 2014 Elsevier Ltd. All rights reserved.
出版日期: 2014-10-22
卷号: 55, 期号:43, 页码:5960-5962
DOI标识: 10.1016/j.tetlet.2014.08.110
语种: 英语
收录类别: SCI ; IC
学科分类: Chemistry
ISSN号: 0040-4039
Citation statistics:
内容类型: 期刊论文
URI标识: http://ir.kib.ac.cn/handle/151853/18391
Appears in Collections:植物化学与西部植物资源持续利用国家重点实验室_期刊论文

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作者单位: 1.Yunnan Univ, Sch Chem Sci & Technol, Key Lab Med Chem Nat Resources, Minist Educ, Kunming 650091, Peoples R China
2.Chinese Acad Sci, Kunming Inst Bot, State Key Lab Phytochem & Plant Resources West Ch, Kunming 650201, Peoples R China
3.Univ Chinese Acad Sci, Beijing 100049, Peoples R China

Recommended Citation:
Li,Liang-Qun;Li,Ming-Ming;Chen,Dong;Liu,Hao-Miao;Geng,Hui-Chun;Lin,Jun;Qin,Hong-Bo.Catalytic asymmetric formal total synthesis of (+)-dichroanone and (+)-taiwaniaquinone H,TETRAHEDRON LETTERS,2014,55(43):5960-5962
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